Underground hydrogen storage (UHS) has emerged as a significant focus for the energy transition from fossil fuels to renewable energy. Saline aquifers, akin to those used in geological CO2 storage, are proposed due to their potential as reservoirs for hydrogen injection and withdrawal over extended periods. Modeling the drainage and imbibition processes at the reservoir scale is critical for efficient UHS implementation. To address the excessive computational costs of three-dimensional simulations over hundreds of cycles, low-order models such as the Vertical Equilibrium (VE) models offer practicality. This study centers on the VE model’s applicability to predict hydrogen plume shapes during a single injection and withdrawal cycle, considering varying viscous, capillary, and buoyancy forces, captured by Capillary number (Ca) and Bond number (Bo). Examining Ca values from 1.5 × 10−9 to 1.5 × 10−7 and Bo numbers from 0.1 to 0.3, we compared VE results to a 2D two-phase simulation, serving as the reference solution. For small Ca, the VE method accurately predicted both vertical and horizontal hydrogen plume distributions, although it occasionally overestimated lateral spread at high injection rates. As the vertical permeability and Bo increase, the VE predictions become more aligned with the reference solution. This is because greater density-driven flow and improved vertical connectivity make the phase segregation easier. Our study also demonstrated the VE model’s promising performance in hydrogen recovery during withdrawal at small Ca and large Bo.
%0 Journal Article
%1 vahabzadeh2025
%A Vahabzadeh, Ehsan
%A Buntic, Ivan
%A Nazari, Farzaneh
%A Flemisch, Bernd
%A Helmig, Rainer
%A Niasar, Vahid
%D 2025
%J International Journal of Hydrogen Energy
%K PN5-2A PN5 PN5-2(II) EXC2075 selected
%P 790-805
%R https://doi.org/10.1016/j.ijhydene.2025.01.201
%T Applicability of the Vertical Equilibrium model to underground hydrogen injection and withdrawal
%U https://www.sciencedirect.com/science/article/pii/S036031992500223X
%V 106
%X Underground hydrogen storage (UHS) has emerged as a significant focus for the energy transition from fossil fuels to renewable energy. Saline aquifers, akin to those used in geological CO2 storage, are proposed due to their potential as reservoirs for hydrogen injection and withdrawal over extended periods. Modeling the drainage and imbibition processes at the reservoir scale is critical for efficient UHS implementation. To address the excessive computational costs of three-dimensional simulations over hundreds of cycles, low-order models such as the Vertical Equilibrium (VE) models offer practicality. This study centers on the VE model’s applicability to predict hydrogen plume shapes during a single injection and withdrawal cycle, considering varying viscous, capillary, and buoyancy forces, captured by Capillary number (Ca) and Bond number (Bo). Examining Ca values from 1.5 × 10−9 to 1.5 × 10−7 and Bo numbers from 0.1 to 0.3, we compared VE results to a 2D two-phase simulation, serving as the reference solution. For small Ca, the VE method accurately predicted both vertical and horizontal hydrogen plume distributions, although it occasionally overestimated lateral spread at high injection rates. As the vertical permeability and Bo increase, the VE predictions become more aligned with the reference solution. This is because greater density-driven flow and improved vertical connectivity make the phase segregation easier. Our study also demonstrated the VE model’s promising performance in hydrogen recovery during withdrawal at small Ca and large Bo.
@article{vahabzadeh2025,
abstract = {Underground hydrogen storage (UHS) has emerged as a significant focus for the energy transition from fossil fuels to renewable energy. Saline aquifers, akin to those used in geological CO2 storage, are proposed due to their potential as reservoirs for hydrogen injection and withdrawal over extended periods. Modeling the drainage and imbibition processes at the reservoir scale is critical for efficient UHS implementation. To address the excessive computational costs of three-dimensional simulations over hundreds of cycles, low-order models such as the Vertical Equilibrium (VE) models offer practicality. This study centers on the VE model’s applicability to predict hydrogen plume shapes during a single injection and withdrawal cycle, considering varying viscous, capillary, and buoyancy forces, captured by Capillary number (Ca) and Bond number (Bo). Examining Ca values from 1.5 × 10−9 to 1.5 × 10−7 and Bo numbers from 0.1 to 0.3, we compared VE results to a 2D two-phase simulation, serving as the reference solution. For small Ca, the VE method accurately predicted both vertical and horizontal hydrogen plume distributions, although it occasionally overestimated lateral spread at high injection rates. As the vertical permeability and Bo increase, the VE predictions become more aligned with the reference solution. This is because greater density-driven flow and improved vertical connectivity make the phase segregation easier. Our study also demonstrated the VE model’s promising performance in hydrogen recovery during withdrawal at small Ca and large Bo.},
added-at = {2025-02-28T16:06:55.000+0100},
author = {Vahabzadeh, Ehsan and Buntic, Ivan and Nazari, Farzaneh and Flemisch, Bernd and Helmig, Rainer and Niasar, Vahid},
biburl = {https://puma.ub.uni-stuttgart.de/bibtex/2c4c42d39d896fc24cd411f864faa64c6/exc2075},
doi = {https://doi.org/10.1016/j.ijhydene.2025.01.201},
interhash = {325a5a872daf1571cc9f8c84c93086bb},
intrahash = {c4c42d39d896fc24cd411f864faa64c6},
issn = {0360-3199},
journal = {International Journal of Hydrogen Energy},
keywords = {PN5-2A PN5 PN5-2(II) EXC2075 selected},
pages = {790-805},
timestamp = {2025-02-28T16:06:55.000+0100},
title = {Applicability of the Vertical Equilibrium model to underground hydrogen injection and withdrawal},
url = {https://www.sciencedirect.com/science/article/pii/S036031992500223X},
volume = 106,
year = 2025
}
