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Crucial Role of Cu-S Bonding for Structural Changes Accompanying the Reversible CuI/CuII Transition in an Unrestrained Cu(N$\cap$S)2 Coordination Arrangement. An Experimental and DFT Study. Inorganic Chemistry, (39)21:4731--4734, 2000. [PUMA: benzimidazole complex complex;electrochem copper electrochem;copper electrochem;crystal methylthiomethyl methylthiomethylbenzimidazole prepn redox structure]