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Single-molecule scale magnetic resonance spectroscopy using quantum diamond sensors

, , , , and . Rev. Mod. Phys., 96 (2): 025001 (May 2024)
DOI: 10.1103/RevModPhys.96.025001

Abstract

Nitrogen-vacancy centers in diamond are sensitive to magnetic fields, and a single center permits detection of electron and nuclear spins and imaging of single molecules in its vicinity. This article reviews the achievements of advanced methods to obtain spectral and spatial resolution and it points to technical problems that remain to be solved for widespread and multidisciplinary adoption of single-molecule magnetic resonance spectroscopy.

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