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Es zeigt sich, dass die Entwicklung auf dem Sektor der Personennormdateien (authorithy records) mittels VIAF und ISNI auf einem guten Wege ist. Bei der notwendigen Zusammenführung der bisherigen Autoren-Identifikatoren in einem übergeordneten System könnte der neuen ORCID-Initiative große Bedeutung zukommen.", "bibtexKey": "pai2010" } , { "type" : "Publication", "id" : "https://puma.ub.uni-stuttgart.de/bibtex/24d706dcb4a19a406cc9383fec48be027/huebleriac", "tags" : [ "EPR","complex","complex;UV","complex;spin","density","g","multifrequency","organo","persistent","radical","rhenium","spectra","tensor","visible" ], "intraHash" : "4d706dcb4a19a406cc9383fec48be027", "interHash" : "171b2796c8cc6986ef821d23de1ae9a2", "label" : "Multifrequency EPR Study and Density Functional g-Tensor Calculations of Persistent Organorhenium Radical Complexes", "user" : "huebleriac", "description" : "", "date" : "2022-06-15 11:26:56", "changeDate" : "2022-06-15 09:26:56", "count" : 3, "pub-type": "article", "journal": "Journal of the American Chemical Society", "year": "2002", "url": "", "author": [ "Stephanie Frantz","Heiko Hartmann","Natasa Doslik","Matthias Wanner","Wolfgang Kaim","Hans-Juergen Kuemmerer","Gert Denninger","Anne-Laure Barra","Carole Duboc-Toia","Jan Fiedler","Ilaria Ciofini","Christian Urban","Martin. Kaupp" ], "authors": [ {"first" : "Stephanie", "last" : "Frantz"}, {"first" : "Heiko", "last" : "Hartmann"}, {"first" : "Natasa", "last" : "Doslik"}, {"first" : "Matthias", "last" : "Wanner"}, {"first" : "Wolfgang", "last" : "Kaim"}, {"first" : "Hans-Juergen", "last" : "Kuemmerer"}, {"first" : "Gert", "last" : "Denninger"}, {"first" : "Anne-Laure", "last" : "Barra"}, {"first" : "Carole", "last" : "Duboc-Toia"}, {"first" : "Jan", "last" : "Fiedler"}, {"first" : "Ilaria", "last" : "Ciofini"}, {"first" : "Christian", "last" : "Urban"}, {"first" : "Martin.", "last" : "Kaupp"} ], "volume": "124","number": "35","pages": "10563--10571","abstract": "The dinuclear radical anion complexes (μ-L)[Re(CO)3Cl]2.bul.-, L = 2,2'-azobispyridine (abpy) and 2,2'-azobis(5-chloropyrimidine) (abcp), were studied by EPR at 9.5, 94, 230, and 285 GHz (abpy complex) and at 9.5 and 285 GHz (abcp complex). Whereas the X-band measurements yielded only the isotropic metal hyperfine coupling of the 185,187Re isotopes, the high-frequency EPR expts. in glassy frozen CH2Cl2/toluene soln. revealed the g components. Both the a(185,187Re) value and the g anisotropy, g1 - g3, are larger for the abcp complex, which contains the better p-accepting bridging ligand. Confirmation for this comes also from IR and UV/visible spectroscopy of the new (μ-abcp)[Re(CO)3Cl]2o/.bul.-/2- redox system. The g values are reproduced reasonably well by d. functional calcns. which confirm higher metal participation at the singly occupied MO and therefore larger contributions from the metal atoms to the g anisotropy in abcp systems compared to abpy complexes. Addnl. calcns. for systems (μ-abcp)[M(CO)3X]2.bul.- (M = Tc or Re and X = Cl, and X = F, Cl, or Br with M = Re) provided further insight into the relation between spin d. distribution and g anisotropy. 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Kaupp" ], "authors": [ {"first" : "Stephanie", "last" : "Frantz"}, {"first" : "Heiko", "last" : "Hartmann"}, {"first" : "Natasa", "last" : "Doslik"}, {"first" : "Matthias", "last" : "Wanner"}, {"first" : "Wolfgang", "last" : "Kaim"}, {"first" : "Hans-Juergen", "last" : "Kuemmerer"}, {"first" : "Gert", "last" : "Denninger"}, {"first" : "Anne-Laure", "last" : "Barra"}, {"first" : "Carole", "last" : "Duboc-Toia"}, {"first" : "Jan", "last" : "Fiedler"}, {"first" : "Ilaria", "last" : "Ciofini"}, {"first" : "Christian", "last" : "Urban"}, {"first" : "Martin.", "last" : "Kaupp"} ], "volume": "124","number": "35","pages": "10563--10571","abstract": "The dinuclear radical anion complexes (μ-L)[Re(CO)3Cl]2.bul.-, L = 2,2'-azobispyridine (abpy) and 2,2'-azobis(5-chloropyrimidine) (abcp), were studied by EPR at 9.5, 94, 230, and 285 GHz (abpy complex) and at 9.5 and 285 GHz (abcp complex). Whereas the X-band measurements yielded only the isotropic metal hyperfine coupling of the 185,187Re isotopes, the high-frequency EPR expts. in glassy frozen CH2Cl2/toluene soln. revealed the g components. Both the a(185,187Re) value and the g anisotropy, g1 - g3, are larger for the abcp complex, which contains the better p-accepting bridging ligand. Confirmation for this comes also from IR and UV/visible spectroscopy of the new (μ-abcp)[Re(CO)3Cl]2o/.bul.-/2- redox system. The g values are reproduced reasonably well by d. functional calcns. which confirm higher metal participation at the singly occupied MO and therefore larger contributions from the metal atoms to the g anisotropy in abcp systems compared to abpy complexes. Addnl. calcns. for systems (μ-abcp)[M(CO)3X]2.bul.- (M = Tc or Re and X = Cl, and X = F, Cl, or Br with M = Re) provided further insight into the relation between spin d. distribution and g anisotropy. [on SciFinder(R)]", "issn" : "0002-7863", "doi" : "10.1021/ja025829n", "bibtexKey": "Frantz.2002" } , { "type" : "Publication", "id" : "https://puma.ub.uni-stuttgart.de/bibtex/2e5edd10266c5e377122b0c2be4432ca0/steenweg2", "tags" : [ "DAI","author","authority","autor","digital","gnd","ident","identification","isni","myown","orcid","pai","persistent","pnd","publication","publikationsmanagement","publikationswesen","recordsifikation","viaf" ], "intraHash" : "e5edd10266c5e377122b0c2be4432ca0", "interHash" : "ada56d12f3dacd95666004f9ce312e0a", "label" : "Eindeutige Autoren-Identifikation \u2013 (PAI \u2013 Persistent Author Identification) \u2013 Versuch einer Annäherung", "user" : "steenweg2", "description" : "", "date" : "2016-01-27 23:20:44", "changeDate" : "2022-08-24 20:28:30", "count" : 5, "pub-type": "article", "journal": "ABI-Technik", "year": "2010", "url": "https://doi.org/10.1515/ABITECH.2010.30.4.240", "author": [ "Helge Steenweg" ], "authors": [ {"first" : "Helge", "last" : "Steenweg"} ], "volume": "30","number": "4","pages": "240-251.","abstract": "Im vorliegenden Beitrag wird die Notwendigkeit einer eindeutigen Autorenidentifikation (Persistant Author Identification - PAI) diskutiert und die bisher vorhandenen fachlichen, nationalen, überregionalen und kommerziellen Ansätze vorgestellt und erläutert. Es zeigt sich, dass die Entwicklung auf dem Sektor der Personennormdateien (authorithy records) mittels VIAF und ISNI auf einem guten Wege ist. Bei der notwendigen Zusammenführung der bisherigen Autoren-Identifikatoren in einem übergeordneten System könnte der neuen ORCID-Initiative große Bedeutung zukommen.", "bibtexKey": "pai2010" } ] }